| Movie | 1992 | Unforgiven | 'Little' Bill Daggett | |
| Movie | 1997 | Absolute Power | President Richmond | |
| Movie | 1967 | Bonnie and Clyde | Buck Barrow | |
| Movie | 1971 | The French Connection | Jimmy Doyle | |
| Movie | 1972 | The Poseidon Adventure | Reverend Scott | |
| Movie | 1974 | The Conversation | Harry Caul | |
| Movie | 1988 | Mississippi Burning | Agent Rupert Anderson | |
| Movie | 1974 | Young Frankenstein | Blindman | |
| Movie | 2000 | Under Suspicion | Henry Hearst | |
| Movie | 1987 | No Way Out | Defense Secretary David Brice | |
| Movie | 1978 | Superman | Lex Luthor | |
| Movie | 2000 | The Replacements | Jimmy McGinty | |
| Movie | 1975 | French Connection II | "Popeye" Doyle | |
| Movie | 2001 | Heartbreakers | William B. Tensy | |
| Movie | 1996 | The Birdcage | Senator Kevin Keeley | |
| Movie | 2001 | Heist | Joe Moore | |
| Movie | 1977 | A Bridge Too Far | Maj. Gen. Stanislaw F. Sosabowski | |
| Movie | 1986 | Hoosiers | Coach Norman Dale | |
| Movie | 1996 | Extreme Measures | Dr. Lawrence Myrick | |
| Movie | 1987 | Superman IV: The Quest for Peace | Lex Luthor | |
| Movie | 2001 | The Mexican | Arnold Margolese | |
| Movie | 2003 | Runaway Jury | Rankin Fitch | |
| Movie | 1990 | Postcards from the Edge | Lowell Kolchek | |
| Movie | 1988 | Another Woman | Larry | |
| Movie | 1973 | Scarecrow | Max Millan | |
| Movie | 2001 | Behind Enemy Lines | Admiral Leslie Reigart, Commander Adriatic Battle Group | |
| Movie | 1990 | Narrow Margin | Robert Caulfield | |
| Movie | 1985 | Target | Walter Lloyd | |
| Movie | 1995 | Get Shorty | Harry Zimm | |
| Movie | 1996 | The Chamber | Sam Cayhall | |
| Movie | 1989 | The Package | Sgt. Johnny Gallagher | |
| Movie | 1968 | The Split | Lt. Walter Brill | |
| Movie | 1980 | Superman II | Lex Luthor | |
| Movie | 1990 | Loose Cannons | MacArthur Stern | |
| Movie | 1977 | The Domino Principle | Tucker | |
| Movie | 1975 | Night Moves | Harry Moseby | |
| Movie | 1995 | The Quick and the Dead | John Herod | |
| Movie | 1991 | Company Business | Sam Boyd | |
| Movie | 1994 | Wyatt Earp | Nicholas Earp | |
| Movie | 1977 | March or Die | Major William Sherman Foster | |
| Movie | 1995 | Crimson Tide | Captain Franklin "Frank" Ramsey | |
| Movie | 1998 | Antz | General Mandible (voice) | |
| Movie | 2001 | The Royal Tenenbaums | Royal Tenenbaum | |
| Movie | 1998 | Twilight | Jack Ames | |
| Movie | 1969 | Downhill Racer | Eugene Claire | |
| Movie | 1975 | Bite the Bullet | Sam Clayton | |
| Movie | 1998 | Enemy of the State | Brill | |
| Movie | 1983 | Uncommon Valor | Col. Cal Rhodes | |
| Movie | 1983 | Under Fire | Alex Grazier | |
| Movie | 1972 | Prime Cut | Mary Ann | |
| Movie | 1969 | Marooned | Buzz Lloyd | |
| Movie | 1993 | Geronimo: An American Legend | Brig. Gen. George Crook | |
| Movie | 1988 | Full Moon in Blue Water | Floyd | |
| Movie | 1966 | Hawaii | John Whipple | |
| Movie | 1964 | Lilith | Norman | |
| Movie | 1988 | Bat★21 | Lt. Col. Iceal Hambleton | |
| Movie | 1993 | The Firm | Avery Tolar | |
| Movie | 1991 | Class Action | Jedediah Tucker Ward | |
| Movie | 1983 | Eureka | Jack McCann | |
| Movie | 1971 | The Hunting Party | Brandt Ruger | |
| Movie | 1969 | The Gypsy Moths | Joe Browdy | |
| Movie | 2004 | Welcome to Mooseport | Monroe Cole | |
| Movie | 1986 | Power | Wilfred Buckley | |
| Movie | 1981 | Reds | Pete van Wherry | |
| Movie | 1983 | Misunderstood | Ned Rawley | |
| Movie | 1971 | Cisco Pike | Officer Leo Holland | |
| Movie | 1970 | I Never Sang for My Father | Gene Garrison | |
| Movie | 1988 | Split Decisions | Dan McGuinn | |
| Movie | 1969 | Riot | Red Fraker | |
| Movie | 2001 | With the Filmmaker: Wes Anderson | Self | |
| Movie | 1975 | Lucky Lady | Kibby | |
| Movie | 1974 | Zandy's Bride | Zandy Allen | |
| Movie | 2004 | Imaginary Witness: Hollywood and the Holocaust | Narrator | |
| Movie | 1985 | Twice in a Lifetime | Harry MacKenzie | |
| Movie | 1981 | All Night Long | George Dupler | |
| Movie | 2008 | Revolution! The Making of 'Bonnie and Clyde' | Self | |
| Movie | 1994 | Shurtleff on Acting | Self | |
| Movie | 1971 | Doctors' Wives | Dave Randolph | |
| Movie | 2001 | Once Upon a Time: The Super Heroes | Lex Luthor (archive footage) | |
| Movie | 1967 | A Covenant with Death | Harmsworth | |
| Movie | 1997 | Sports on the Silver Screen | Self (archive footage) | |
| Movie | 2001 | Heroes of Iwo Jima | Self - Host/Narrator | |
| Movie | 2019 | Sacheen: Breaking the Silence | Self (archive footage) | |
| Movie | 2017 | Pattern Recognition | Self (archive footage) | |
| Movie | 1969 | The Sky Divers | Self | |
| Movie | 1967 | First to Fight | Sergeant Tweed | |
| Movie | 2001 | Making the Connection: Untold Stories of The French Connection | Self | |
| Movie | 2000 | Clint Eastwood: Out of the Shadows | Self | |
| Movie | 2013 | Eastwood Directs: The Untold Story | Self | |
| Movie | 1967 | Banning | Tommy Del Gaddo | |
| Movie | 1968 | Shadow on the Land | Rev. Thomas Davis | |
| Movie | 2009 | I Knew It Was You: Rediscovering John Cazale | Self | |
| Movie | 1999 | Hitchcock, Selznick and the End of Hollywood | Narrator (voice) | |
| Movie | 2001 | Taking Flight: The Development of 'Superman' | Self | |
| Movie | 1982 | The Making of 'Superman: The Movie' | Self | |
| Movie | 1983 | The Making of 'Superman II' | Self | |
| Movie | 2001 | Making 'Superman': Filming the Legend | Self | |
| Movie | 2002 | Page to Screen: 'The Silence of the Lambs' | Self | |
| Movie | 1961 | Mad Dog Coll | Cop (uncredited) | |
| Movie | 2017 | We, the Marines | Self - Narrator (voice) | |
| Movie | 2005 | Shipibo Konibo: A Rite of Passage | Narrator (voice) | |
| Movie | 1978 | Formula 1 - Speed fever | Self | |
| Movie | 2006 | Superman II: The Richard Donner Cut | Lex Luthor | |
| Movie | 1992 | Earth and the American Dream | Reader (voice) | |
| Movie | 2002 | Eastwood & Co.: Making 'Unforgiven' | Self | |
| Movie | 2002 | All on Accounta Pullin' a Trigger | Self | |
| Movie | 1996 | Making Frankensense of Young Frankenstein | Blind Man (archive footage) | |
| Movie | 1983 | Two of a Kind | God (voice) (uncredited) | |
| Movie | 1994 | Clint Eastwood: The Man from Malpaso | Self | |
| Movie | 2000 | The Poughkeepsie Shuffle: Tracing 'The French Connection' | Self | |
| Movie | 2021 | Quentin Tarantino: From a Movie Buff to a Hollywood Legend | Self (archive footage) | |
| Movie | 2001 | Will Shuster's Zozobra™ de Santa Fe | Himself/Narrator | |
| Movie | 1992 | Eastwood & Co.: Making 'Unforgiven' | Self | |
| Movie | 1973 | On the Road with: Scarecrow | Himself | |
| Movie | 1995 | The Making of 'Crimson Tide' | Self | |
| Movie | 2016 | The Unknown Flag Raiser of Iwo Jima | Self - Narrator | |
| Movie | 2025 | The Last Days of Gene Hackman: ABC News Special | Self (Archival Footage) | |
| Movie | 2014 | Electric Boogaloo: The Wild, Untold Story of Cannon Films | Lex Luthor (archive footage) (uncredited) | |
| TV Show | 1985 | Larry King Live | Self | 1 |
| TV Show | 1994 | Inside the Actors Studio | Self | 1 |
| TV Show | 1965 | The F.B.I. | Herb Kenyon | 1 |
| TV Show | 1978 | The South Bank Show | Self | 1 |
| TV Show | 1958 | Naked City | Mr. Jasper | 1 |
| TV Show | 1963 | East Side/West Side | | 1 |
| TV Show | 1968 | Rowan & Martin's Laugh-In | Self | 2 |
| TV Show | 1961 | The Defenders | Stanley McGuirk | 2 |
| TV Show | 1953 | The United States Steel Hour | | 5 |
| TV Show | 1966 | CBS Playhouse | | 1 |
| TV Show | 1961 | The DuPont Show of the Week | Douglas McCann | 1 |
| TV Show | 1999 | The Directors | Self | 1 |
| TV Show | 1977 | The Hollywood Greats | | 1 |
| TV Show | 1953 | The Oscars | Self | 5 |
| TV Show | 1966 | Hawk | | 1 |
| TV Show | 1961 | Tallahassee 7000 | Joe Lawson | 1 |
| TV Show | 1965 | The Trials of O'Brien | Roger Nathan | 1 |
| TV Show | 1962 | The Tonight Show Starring Johnny Carson | Self | 6 |
| TV Show | 2006 | America's Game: The Super Bowl Champions | Self - Narrator (voice) | 4 |
| TV Show | 1973 | The American Film Institute Salute to ... | Self | 1 |
| TV Show | 2007 | Diners, Drive-Ins and Dives | Self | 1 |
| TV Show | 1971 | V.I.P. Schaukel | Self | 1 |
| TV Show | 1986 | American Masters | Self | 1 |
| TV Show | 1961 | The Mike Douglas Show | Self | 7 |
| TV Show | 1981 | Entertainment Tonight | Self | 1 |
| TV Show | 1967 | The Invaders | Tom Jessup | 1 |
| TV Show | 2023 | The Playboy Murders | Self (archive footage) | 1 |
| TV Show | 1944 | Golden Globe Awards | Self - Nominee | 1 |
| TV Show | 1944 | Golden Globe Awards | Self - Presenter | 2 |
| TV Show | 1944 | Golden Globe Awards | Self - Cecil B. DeMille Award Recipient | 1 |
| TV Show | 1960 | Route 66 | Motorist | 1 |
| TV Show | 1944 | Golden Globe Awards | Self - Nominee / Presenter | 1 |
| TV Show | 1956 | Tony Awards | Self - Presenter | 1 |
| TV Show | 1974 | Dinah! | Self | 1 |
| TV Show | 1962 | The Merv Griffin Show | Self | 5 |
| TV Show | 1971 | Film '72 | Self | 2 |
